[Code of Federal Regulations]
[Title 40, Volume 14]
[Revised as of July 1, 2003]
From the U.S. Government Printing Office via GPO Access
[CITE: 40CFR79.61]
[Page 541-551]
TITLE 40--PROTECTION OF ENVIRONMENT
CHAPTER I--ENVIRONMENTAL PROTECTION AGENCY (CONTINUED)
PART 79--REGISTRATION OF FUELS AND FUEL ADDITIVES--Table of Contents
Subpart F--Testing Requirements for Registration
Sec. 79.61 Vehicle emissions inhalation exposure guideline.
(a) Purpose. This guideline provides additional information on
methodologies required to conduct health effects tests involving
inhalation exposures to vehicle combustion emissions from fuels or fuel/
additive mixtures. Where this guideline and the other health effects
testing guidelines in 40 CFR 79.62 through 79.68 specify differing
values
[[Page 542]]
for the same test parameter, the specifications in the individual health
test guideline shall prevail for that health effect endpoint.
(b) Definitions. For the purposes of this section the following
definitions apply.
Acute inhalation study means a short-term toxicity test
characterized by a single exposure by inhalation over a short period of
time (at least 4 hours and less than 24 hours), followed by at least 14
days of observation.
Aerodynamic diameter means the diameter of a sphere of unit density
that has the same settling velocity as the particle of the test
substance. It is used to compare particles of different sizes, densities
and shapes, and to predict where in the respiratory tract such particles
may be deposited. It applies to the size of aerosol particles.
Chronic inhalation study means a prolonged and repeated exposure by
inhalation for the life span of the test animal; technically, two years
in the rat.
Concentration means an exposure level. Exposure is expressed as
weight or volume of test aerosol/substance per volume of air, usually
mg/m3 or as parts per million (ppm) over a given time period.
Micrograms per cubic meter ([mu]g/m3) or parts per billion
may be appropriate, as well.
Cumulative toxicity means the adverse effects of repeated exposures
occurring as a result of prolonged action or increased concentration of
the administered test substance or its metabolites in the susceptible
tissues.
Inhalable diameter means that aerodynamic diameter of a particle
which is considered to be inhalable for the organism. It is used to
refer to particles which are capable of being inhaled and may be
deposited anywhere within the respiratory tract from the trachea to the
alveoli.
Mass median aerodynamic diameter (MMAD) means the calculated
aerodynamic diameter, which divides the particles of an aerosol in half
based on the mass of the particles. Fifty percent of the particles in
mass will be larger than the median diameter, and fifty percent will be
smaller than the median diameter. MMAD describes the particle
distribution of any aerosol based on the weight and size of the
particles. MMAD and the geometric standard deviation describe the
particle-size distribution.
Material safety data sheet (MSDS) means documentation or information
on the physical, chemical, and hazardous characteristics of a given
chemical, usually provided by the product's manufacturer.
Reynolds number means a dimensionless number that is proportional to
the ratio of inertial forces to frictional forces acting on a fluid. It
quantitatively provides a measure of whether flow is laminar or
turbulent. A fluid traveling through a pipe is fully developed into a
laminar flow for a Reynolds number less than 2000, and fully developed
into a turbulent flow for a Reynolds number greater than 4000.
Subacute inhalation toxicity means the adverse effects occurring as
a result of the repeated daily exposure of experimental animals to a
chemical by inhalation for part (less than 10 percent) of a lifespan;
generally, less than 90 days.
Subchronic inhalation study means a repeated exposure by inhalation
for part (approximately 10 percent) of a life span of the exposed test
animal.
Toxic effect means an adverse change in the structure or function of
an experimental animal as a result of exposure to a chemical substance.
(c) Principles and design criteria of inhalation exposure systems.
Proper conduct of inhalation toxicity studies of the emissions of fuels
and additive/fuel mixtures requires that the exposure system be designed
to ensure the controlled generation of the exposure atmosphere, the
adequate dilution of the test emissions, delivery of the diluted
exposure atmosphere to the test animals, and use of appropriate exposure
chamber systems selected to meet criteria for a given exposure study.
(1) Emissions generation. Emissions shall be generated according to
the specifications in 40 CFR 79.57.
(2) Dilution and delivery systems. (i) The delivery system is the
means used to transport the emissions from the generation system to the
exposure system. The dilution system is generally a component of the
delivery system.
(ii) Dilution provides control of the emissions concentration
delivered to
[[Page 543]]
the exposure system, serving the function of diluting the associated
combustion gases, such as carbon monoxide, carbon dioxide, nitrogen
oxides, sulfur dioxide and other noxious gases and vapors, to levels
that will ensure that there are no significant or measurable responses
in the test animals as a result of exposure to the combustion gases. The
formation of particle species is strongly dependent on the dilution
rate, as well.
(iii) The engine exhaust system shall connect to the first-stage-
dilution section at 90 deg. to the axis of the dilution section. This is
then connected to a right angle elbow on the center line of the dilution
section. Engine emissions are injected through the elbow so that exhaust
flow is concurrent to dilution flow.
(iv) Materials. In designing the dilution and delivery systems, the
use of plastic, e.g., PVC and similar materials, copper, brass, and
aluminum pipe and tubing shall be avoided if there exists a possibility
of chemical reaction occurring between emissions and tubing. Stainless
steel pipe and tubing is recommended as the best choice for most
emission dilution and delivery applications, although glass and teflon
may be appropriate, as well.
(v) Flow requirements. (A) Conduit for dilute raw emissions shall be
of such dimensions as to provide residence times for the emissions on
the order of less than one second to several seconds before the
emissions are further diluted and introduced to the test chambers. With
the high flow rates in the dilute raw emissions conduit, it will be
necessary to sample various portions of the dilute emissions for
delivering differing concentrations to the test chambers. The unused
portions of the emissions stream are normally exhausted to the
atmosphere outside of the exposure facility.
(B) Dimensions of the dilute raw exhaust conduit shall be such that,
at a minimum, the flow Reynolds number is 70,000 or greater (see Mokler,
et al., 1984 in paragraph (f)(13) of this section). This will maintain
highly turbulent flow conditions so that there is more complete mixing
of the exhaust emissions.
(C) Wall losses. The delivery system shall be designed to minimize
wall losses. This can be done by sizing the tubing or pipe to maintain
laminar flow of the diluted emissions to the exposure chamber. A flow
Reynolds number of 1000-3000 will ensure minimal wall losses. Also, the
length of and number and degree of bends in the delivery lines to the
exposure chamber system shall be minimized.
(D) Whole-body exposure vs. nose-only exposure delivery systems.
Flow rates through whole-body chamber systems are of the order of 100
liters per minute to 500 liters per minute. Nose-only systems are on the
order of less than 50 liters per minute. To maintain laminar flow
conditions, the principles described in paragraph (c)(2)(v)(C) of this
section apply to both systems.
(vi) Dilution requirements. (A) To maintain the water vapor, and
dissolved organic compounds, in the raw exhaust emissions stream, a
manufacturer/tester will initially dilute one part emissions with a
minimum of five parts clean, filtered air (see Hinners, et al., 1979 in
paragraph (f)(11) of this section). Depending on the water vapor content
of a particular fuel/additive mixture's combustion emissions and the
humidity of the dilution air, initial exhaust dilutions as high as 1:15
or 1:20 may be necessary to maintain the general character of the
exhaust as it cools, e.g., M100. At this point, it is expected that the
exhaust stream would be further diluted to more appropriate levels for
rodent health effects testing.
(B) A maximum concentration (minimum dilution) of the raw exhaust
going into the test animal cages is anticipated to lie in the range
between 1:5 and 1:50 exhaust emissions to clean, filtered air. The
minimum concentration (maximum dilution) of raw exhaust for health
effects testing is anticipated to be in range between 1:100 and 1:150.
Individual manufacturers will treat these ranges as approximations only
and will determine the optimum range of emission concentrations to
elicit effects in Tier 2 health testing for their particular fuel/fuel
additive mixture.
(3) Exposure chamber systems--(i) Referenced Guidelines. (A) The
U.S. Department of Health and Human Services
[[Page 544]]
``Guide for the Care and Use of Laboratory Animals'' (Guide), 1985 cited
in paragraph (c)(3)(ii)(A)(4), and in paragraphs (d)(2)(i), (d)(2)(ii),
(d)(2)(iii), (d)(4)(ii), and (d)(4)(iii) of this section, has been
incorporated by reference.
(B) This incorporation by reference was approved by the Director of
the Federal Register in accordance with 5 U.S.C. 552(a) and 1 CFR part
51. Copies may be purchased from the Superintendent of Documents, U.S.
Government Printing Office, Washington, DC 20402. Copies may be
inspected at U.S. EPA, OAR, 401 M Street SW, Washington, DC 20460 or at
the Office of the Federal Register, 800 North Capitol Street NW., suite
700, Washington, DC.
(ii) Exposure chambers. There are two basic types of dynamic
inhalation exposure chambers, whole-body chambers and nose-/head-only
exposure chambers (see Cheng and Moss, 1989 in paragraph (f)(8) of this
section).
(A) Whole-body chambers. (1) The flow rate through a chamber shall
be maintained at 15 air changes per hour.
(2) The chambers are usually maintained at a slightly negative
pressure (0.5 to 1.5 inch of water) to prevent leakage of test substance
into the exposure room.
(3) The exposure chamber shall be designed in such a way as to
provide uniform distribution of exposure concentrations in all
compartments (see Cheng et al., 1989 in paragraph (f)(7) of this
section).
(4) Animals are housed in separate compartments inside the chamber,
where the whole surface area of an animal is exposed to the test
material. The spaces required for different animal species shall follow
the Guide. In general, the volume of animal bodies occupy less than 5
percent of the chamber volume.
(B) Head/nose-only exposure chambers. (1) In head/nose-only exposure
chambers, only the head (oronasal) portion of the animal is exposed to
the test material.
(2) The chamber volume and flow rates are much less than in the
whole-body exposure chambers because the subjects are usually restrained
in a tube holder where the animal's breathing can be easily monitored.
The head/nose-only exposure chamber is suitable for short-term exposures
or when use of a small amount of test material is required.
(iii) Since whole-body exposure appears to be the least stressful
mode of exposure, it is the preferred method. In general, head/nose only
exposure, which is sometimes used to avoid concurrent exposure by the
dermal or oral routes, i.e., grooming, is not recommended because of the
stress accompanying the restraining of the animals. However, there may
be specific instances where it may be more appropriate than whole-body
exposure. The tester shall provide justification for its selection.
(d) Inhalation exposure procedures--(1) Animal selection. (i) The
rat is the preferred species for vehicle emission inhalation health
effects testing. Commonly used laboratory strains shall be used. Any
rodent species may be used, but the tester shall provide justification
for the choice of that species.
(ii) Young adult animals, approximately ten weeks of age for the
rat, shall be used. At the commencement of the study, the weight
variation of animals used shall not exceed 20 percent of the
mean weight for each sex. Animals shall be randomly assigned to
treatment and control groups according to their weight.
(iii) An equal number of male and female rodents shall be used at
each concentration level. Situations may arise where use of a single sex
may be appropriate. Females, in general, shall be nulliparous and
nonpregnant.
(iv) The number of animals used at each concentration level and in
the control group(s) depends on the type of study, number of biological
end points used in the toxicity evaluation, the pre-determined
sensitivity of detection and power of significance of the study, and the
animal species. For an acute study, at least five animals of each sex
shall be used in each test group. For both the subacute and subchronic
studies, at least 10 rodents of each sex shall be used in each test
group. For a chronic study, at least 20 male and 20 female rodents shall
be used in each test group.
(A) If interim sacrifices are planned, the number of animals shall
be increased by the number of animals
[[Page 545]]
scheduled to be sacrificed during the course of the study.
(B) For a chronic study, the number of animals at the termination of
the study must be adequate for a meaningful and valid statistical
evaluation of chronic effects.
(v) A concurrent control group is required. This group shall be
exposed to clean, filtered air under conditions identical to those used
for the group exposed to the test atmosphere.
(vi) The same species/strain shall be used to make comparisons
between fuel-only and fuel/additive mixture studies. If another species/
strain is used, the tester shall provide justification for its
selection.
(2) Animal handling and care. (i) A key element in the conduct of
inhalation exposure studies is the proper handling and care of the test
animal population. Therefore, the exposure conditions must conform
strictly with the conditions for housing and animal care and use set
forth in the Guide.
(ii) In whole-body exposure chambers, animals shall be housed in
individual caging. The minimum cage size per animal will be in
accordance with instructions set forth in the Guide.
(iii) Chambers shall be cleaned and maintained in accordance with
recommendations and schedules set forth in the Guide.
(A) Observations shall be made daily with appropriate actions taken
to minimize loss of animals to the study (e.g., necropsy or
refrigeration of animals found dead and isolation or sacrifice of weak
or moribund animals). Exposure systems using head/nose-only exposure
chambers require no special daily chamber maintenance. Chambers shall be
inspected to ensure that they are clean, and that there are no
obstructions in the chamber which would restrict air flow to the
animals. Whole-body exposure chambers will be inspected on a minimum of
twice daily, once before exposures and once after exposures.
(B) Signs of toxicity shall be recorded as they are observed,
including the time of onset, degree, and duration.
(C) Cage-side observations shall include, but are not limited to:
changes in skin, fur, eye and mucous membranes, respiratory, autonomic,
and central nervous systems, somatomotor activity, and behavioral
patterns. Particular attention shall be directed to observation of
tremors, convulsions, salivation, diarrhea, lethargy, sleep, and coma.
(iv) Food and water will be withheld from animals for head/nose-only
exposure systems. For whole-body-exposure systems, water only may be
provided. When the exposure generation system is not operating, food
will be available ad libitum. During operation of the generation system,
food will be withheld to avoid possible contamination by emissions.
(v) At the end of the study period, all survivors in the main study
population shall be sacrificed. Moribund animals shall be removed and
sacrificed when observed.
(3) Concentration levels and selection. (i) In acute and subacute
toxicity tests, at least three exposure concentrations and a control
group shall be used and spaced appropriately to produce test groups with
a range of toxic effects and mortality rates. The data shall be
sufficient to produce a concentration-response curve and permit an
acceptable estimation of the median lethal concentration.
(ii) In subchronic and chronic toxicity tests, testers shall use at
least three different concentration levels, with a control exposure
group, to determine a concentration-response relationship.
Concentrations shall be spaced appropriately to produce test groups with
a range of toxic effects. The concentration-response data may also be
sufficient to determine a NOAEL, unless the result of a limit test
precludes such findings. The criteria for selecting concentration levels
has been published (40 CFR 798.2450 and 798.3260).
(A) The highest concentration shall result in toxic effects but not
produce an incidence of fatalities which would prevent a meaningful
evaluation of the study.
(B) The lowest concentration shall not produce toxic effects which
are directly attributable to the test exposure. Where there is a useful
estimation of human exposure, the lowest concentration shall exceed
this.
[[Page 546]]
(C) The intermediate concentration level(s) shall produce minimal
observable toxic effects. If more than one intermediate concentration
level is used, the concentrations shall be spaced to produce a gradation
of toxic effects.
(D) In the low, intermediate, and control exposure groups, the
incidence of fatalities shall be low to absent, so as not to preclude a
meaningful evaluation of the results.
(4) Exposure chamber environmental conditions. The following
environmental conditions in the exposure chamber are critical to the
maintenance of the test animals: flow; temperature; relative humidity;
lighting; and noise.
(i) Filtered and conditioned air shall be used during exposure, to
dilute the exhaust emissions, and during non- exposure periods to
maintain environmental conditions that are free of trace gases, dusts,
and microorganisms on the test animals. Twelve to fifteen air changes
per hour will be provided at all times to whole-body-exposure chambers.
The minimum air flow rate for head/nose-only exposure chambers will be a
function of the number of animals and the average minute volume of the
animals:
Qminimum(L/min)=2 x number of animals x average minute volume
(see Cheng and Moss, 1989 in paragraph (f)(8) of this section).
(ii) Recommended ranges of temperature for various species are given
in the Guide. The recommended temperature ranges will be used for
establishing temperature conditions of whole-body- exposure chambers.
For rodents in whole-body-exposure chambers, the recommended temperature
is 22 deg.C 2 deg.C and for rabbits, it is 20 deg.C
3 deg.C. Temperature ranges have not been established for
head/nose-only tubes; however, recommended maximum temperature limits
have been established at the Inhalation Toxicology Research Institute
(see Barr, 1988 in paragraph (f)(1) of this section). Maximum
temperature for rats and mice in head/nose-only tubes is 23 deg.C.
(iii) Relative humidity. The relative humidity in the chamber air is
important for heat balance and shall be maintained between 40 percent
and 60 percent, but in certain instances, this may not be practicable.
Testers shall follow Guide recommends for a 30 percent to 70 percent
relative humidity range for rodents in exposure chambers.
(iv) Lighting. Light intensity of 30 foot candles at 3 ft. from the
floor of the exposure facility is recommended (see Rao, 1986 in
paragraph (f)(16) of this section).
(5) Exposure conditions. Unless precluded by the requirements of a
particular test protocol, animal subjects shall be exposed to the test
atmosphere based on a nominal 5-day-per-week regimen, subject to the
following rules:
(i) Each daily exposure must be at least 6 hours plus the time
necessary to build the chamber atmosphere to 90 percent of the target
exposure atmosphere. Interruptions of daily exposures caused by
technical difficulties, if infrequent in occurrence and limited in
duration, may be made up the same day by adding equivalent exposure time
after the technical problem has been corrected and the exposure
atmosphere restored to the required level.
(ii) Normally, no more than two non-exposure days may occur
consecutively during the test period. However, if a third consecutive
non-exposure day should occur due to circumstances beyond the tester's
control, it may be remedied by adding a supplementary exposure day.
Federal and other holidays do not constitute such circumstances.
Whenever possible, a make-up day should be taken at the first
opportunity, i.e., on the next day which would otherwise have been an
intentional non-exposure day. If a compensatory day must be scheduled at
the end of the standard test period, then it may occur either:
(A) Immediately following the last standard exposure day, with no
intervening non-exposure days; or
(B) With up to two intervening non-exposure days, provided that no
fewer than two consecutive compensatory exposure days are completed
before the test is terminated and the animals sacrificed.
(iii) Except as allowed in paragraph (d)(5)(ii)(B) of this section,
in no case shall there be fewer than four exposure days per week at any
time during the test period.
[[Page 547]]
(iv) A nominal 90-day (13-week) subchronic test period shall include
no fewer than 63 total exposure days.
(6) Exposure atmosphere. (i) The exposure atmosphere shall be held
as constant as is practicable and must be monitored continuously or
intermittently, depending on the method of analysis, to ensure that
exposure levels are at the target values or within stated limits during
the exposure period. Sampling methodology will be determined based on
the type of generation system and the type of exposure chamber system
specified for the exposure study.
(A) Integrated samples of test atmosphere aerosol shall be taken
daily during the exposure period from a single representative sample
port in the chamber near the breathing zone of the animals. Gas samples
shall be taken daily to determine concentrations (ppm) of the major
vapor components of the test atmosphere including CO, CO2,
NOX, SO2, and total hydrocarbons.
(B) To ensure that animals in different locations of the chamber
receive a similar exposure atmosphere, distribution of an aerosol or
vapor concentration in exposure chambers can be determined without
animals during the developmental phase of the study, or it can be
determined with animals early in the study. For head/nose-only exposure
chambers, it may not be possible to monitor the chamber distribution
during the exposure, because the exposure port contains the animal.
(C) During the development of the emissions generation system,
particle size analysis shall be performed to establish the stability of
an aerosol concentration with respect to particle size. Over the course
of the exposure, analysis shall be conducted as often as is necessary to
determine the consistency of particle size distribution.
(D) Chamber rise and fall times. The rise time required for the
exposure concentration to reach 90 percent of the stable concentration
after the generator is turned on, and the fall time when the chamber
concentration decreases to 10 percent of the stable concentration after
the generation system is stopped shall be determined in the
developmental phase of the study. Time-integrated samples collected for
calculating exposure concentrations shall be taken after the rise time.
The daily exposure time is exclusive of the rise or the fall time.
(ii) Instrumentation used for a given study will be determined based
on the type of generation system and the type of exposure chamber system
specified for the exposure study.
(A) For exhaust studies, combustion gases shall be sampled by
collecting exposure air in bags and then analyzing the collected air
sample to determine major components of the combustion gas using gas
analyzers. Exposure chambers can also be connected to gas analyzers
directly by using sampling lines and switching valves. Samples can be
taken more frequently using the latter method. Aerosol instruments, such
as photometers, or time-integrated gravimetric determination may be used
to determine the stability of any aerosol concentration in the chamber.
(B) For evaporative emission studies, concentration of fuel vapors
can usually be determined by using a gas chromatograph (GC) and/or
infrared (IR) spectrometry. Grab samples for intermittent sampling can
be taken from the chamber by using bubble samplers with the appropriate
solvent to collect the vapors, or by collecting a small volume of air in
a syringe. Intermediate or continuous monitoring of the chamber
concentration is also possible by connecting the chamber with a GC or IR
detector.
(7) Monitoring chamber environmental conditions may be performed by
a computer system or by exposure system operating personnel.
(i) The flow-metering device used for the exposure chambers must be
a continuous monitoring device, and actual flow measurements must be
recorded at least every 30 minutes. Accuracy must be 5
percent of full scale range. Measurement of air flow through the
exposure chamber may be accomplished using any device that has
sufficient range to accurately measure the air flow for the given
chamber. Types of flow metering devices include rotameters, orifice
meters, venturi meters, critical orifices, and turbinemeters (see
Benedict, 1984 in
[[Page 548]]
paragraph (f)(4) and Spitzer, 1984 in paragraph (f)(17) of this
section).
(ii) Pressure. Pressure measurement may be accomplished using
manometers, electronic pressure transducers, magnehelics, or similar
devices (see Gillum, 1982 in paragraph (f)(10) of this section).
Accuracy of the pressure device must be 5 percent of full
scale range. Pressure measurements must be continuous and recorded at
least every 30 minutes.
(iii) Temperature. The temperature of exposure chambers must be
monitored continuously and recorded at least every 30 minutes.
Temperature may be measured using thermometers, RTD's, thermocouples,
thermistors, or other devices (see Benedict, 1984 in paragraph (f)(4) of
this section). It is necessary to incorporate an alarm system into the
temperature monitoring system. The exposure operators must be notified
by the alarm system when the chamber temperature exceeds 26.7 deg.C (80
deg.F). The exposure must be discontinued and emergency procedures
enacted to immediately reduce temperatures or remove test animals from
high temperature environment when chamber temperatures exceed 29 deg.C.
Accuracy of the temperature monitoring device will be 1
deg.C for the temperature range of 20-30 deg.C.
(iv) Relative humidity. The relative humidity of exposure chambers
must be monitored continuously and recorded at least every 30 minutes.
Relative humidity may be measured using various devices (see Chaddock,
1985 in paragraph (f)(6) of this section).
(v) Lighting shall be measured quarterly, or once at the beginning,
middle, and end of the study for shorter studies.
(vi) Noise level in the exposure chamber(s) shall be measured
quarterly, or once at the beginning, middle, and end of the study for
shorter studies.
(vii) Oxygen content is critical, especially in nose-only chamber
systems, and shall be greater than or equal to 19 percent in the test
cages. An oxygen sensor shall be located at a single position in the
test chamber and a lower alarm limit of 18 percent shall be used to
activate an alarm system.
(8) Safety procedures and requirements. In the case of potentially
explosive test substance concentrations, care shall be taken to avoid
generating explosive atmospheres.
(i) It is mandatory that the upper explosive limit (UEL) and lower
explosive limit (LEL) for the fuel and/or fuel additive(s) that are
being tested be determined. These limits can be found in the material
safety data sheets (MSDS) for each substance and in various reference
texts. The air concentration of the fuel or additive-base fuel mixture
in the generation system, dilution/delivery system, and the exposure
chamber system shall be calculated to ensure that explosive limits are
not present.
(ii) Storage, handling, and use of fuels or fuel/additive mixtures
shall follow guidelines given in 29 CFR 1910.106.
(iii) Monitoring for carbon monoxide (CO) levels is mandatory for
combustion systems. CO shall be continuously monitored in the immediate
area of the engine/vehicle system and in the exposure chamber(s).
(iv) Air samples shall be taken quarterly in the immediate area of
the vapor generation system and the exposure chamber system, or once at
the beginning, middle, and end of the study for shorter studies. These
samples shall be analyzed by methods described in paragraph
(d)(6)(ii)(B) of this section.
(v) With the presence of fuels and/or fuel additives, all electrical
and electronic equipment must be grounded. Also, the dilution/delivery
system and chamber exposure system must be grounded. Guidelines for
grounding are given in 29 CFR 1910.304.
(9) Quality control and quality assurance procedures--(i) Standard
operating procedures (SOPs). SOPs for exposure operations, sampling
instruments, animal handling, and analytical methods shall be written
during the developmental phase of the study.
(ii) Technicians/operators shall be trained in exposure operation,
maintenance, and documentation, as appropriate, and their training shall
be documented.
(iii) Flow meters, sampling instruments, and balances used in the
inhalation experiments shall be calibrated with standards during the
developmental phase to determine their sensitivity, detection limits,
and linearity.
[[Page 549]]
During the exposure period, instruments shall be checked for calibration
and documented to ensure that each instrument still functions properly.
(iv) The mean exposure concentration shall be within 10 percent of
the target concentration on 90 percent or more of exposure days. The
coefficient of variation shall be within 25 percent of target on 90
percent or more of exposure days. For example, a manufacturer might
determine a mean exposure concentration of its product's exposure
emissions by identifying ``marker'' compound(s) typical of the emissions
of the fuel or fuel/additive mixture under study as a surrogate for the
total of individual compounds in those exposure emissions. The
manufacturer would note any concentration changes in the level of the
``marker'' compound(s) in the sample's daily emissions for biological
testing.
(v) The spatial variation of the chamber concentration shall be 10
percent, or less. If a higher spatial variation is observed during the
developmental phase, then air mixing in the chamber shall be increased.
In any case, animals shall be rotated among the various cages in the
exposure chamber(s) to insure each animal's uniform exposure during the
study.
(e) Data and reporting. Data shall be summarized in tabular form,
showing for each group the number of animals at the start of the test,
the number of animals showing lesions, the types of lesions, and the
percentage of animals displaying each type of lesion.
(1) Treatment of results. All observed results, quantitative and
incidental, shall be evaluated by an appropriate statistical method. Any
generally accepted statistical method may be used; the statistical
methods shall be selected during the design of the study.
(2) Evaluation of results. The findings of an inhalation toxicity
study should be evaluated in conjunction with the findings of preceding
studies and considered in terms of the observed toxic effects and the
necropsy and histopathological findings. The evaluation will include the
relationship between the concentration of the test atmosphere and the
duration of exposure, and the severity of abnormalities, gross lesions,
identified target organs, body weight changes, effects on mortality and
any other general or specific toxic effects.
(3) Test conditions. (i) The exposure apparatus shall be described,
including:
(A) The vehicle/engine design and type, the dynamometer, the cooling
system, if any, the computer control system, and the dilution system for
exhaust emission generation;
(B) The evaporative emissions generator model, type, or design and
its dilution system; and
(C) Other test conditions, such as the source and quality of mixing
air, fuel or fuel/additive mixture used, treatment of exhaust air,
design of exposure chamber and the method of housing animals in a test
chamber shall be described.
(ii) The equipment for measuring temperature, humidity, particulate
aerosol concentrations and size distribution, gas analyzers, fuel vapor
concentrations, chamber distribution, and rise and fall time shall be
described.
(iii) Daily exposure results. The daily record shall document the
date, the start and stop times of the exposure, number of samples taken
during the day, daily concentrations determined, calibration of
instruments, and problems encountered during the exposure. The daily
exposure data shall be signed by the exposure operator and reviewed and
signed by the exposure supervisor responsible for the study.
(4) Exposure data shall be tabulated and presented with mean values
and a measure of variability (e.g., standard deviation), and shall
include:
(i) Airflow rates through the inhalation equipment;
(ii) Temperature and humidity of air;
(iii) Chamber concentrations in the chamber breathing zone;
(iv) Concentration of combustion exhaust gases in the chamber
breathing zone;
(v) Particle size distribution (e.g., mass median aerodynamic
diameter and geometric standard deviation from the mean);
(vi) Rise and fall time;
(vii) Chamber concentrations during the non-exposure period; and
(viii) Distribution of test substance in the chamber.
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(5) Animal data. Tabulation of toxic response data by species,
strain, sex and exposure level for:
(i) Number of animals exposed;
(ii) Number of animals showing signs of toxicity; and
(iii) Number of animals dying.
(f) References. For additional background information on this
exposure guideline, the following references should be consulted.
(1) Barr, E.B. (1988) Operational Limits for Temperature and Percent
Oxygen During HM Nose-Only Exposures--Emergency Procedures [interoffice
memorandum]. Albuquerque, NM: Lovelace Inhalation Toxicology Research
Institute; May 13.
(2) Barr, E.B.; Cheng, Y.S.; Mauderly, J.L. (1990) Determination of
Oxygen Depletion in a Nose-Only Exposure Chamber. Presented at: 1990
American Association for Aerosol Research; June; Philadelphia, PA:
American Association for Aerosol Research; abstract no. P2e1.
(3) Barrow, C.S. (1989) Generation and Characterization of Gases and
Vapors. In: McClellan, R.O., Henderson, R.F. ed. Concepts in Inhalation
Toxicology. New York, NY: Hemisphere Publishing Corp., 63-84.
(4) Benedict, R.P. (1984) Fundamentals of Temperature, Pressure, and
Flow Measurements. 3rd ed. New York, NY: John Wiley and Sons.
(5) Cannon, W.C.; Blanton, E.F.; McDonald, K.E. The Flow-Past
Chamber. (1983) An Improved Nose-Only Exposure System for Rodents. Am.
Ind. Hyg. Assoc. J. 44: 923-928.
(6) Chaddock, J.B. ed. (1985) Moisture and humidity. Measurement and
Control in Science and Industry: Proceedings of the 1985 International
Symposium on Moisture and Humidity; April 1985; Washington, D.C.
Research Triangle Park, NC: Instrument Society of America.
(7) Cheng, Y.S.; Barr, E.B.; Carpenter, R.L.; Benson, J.M.; Hobbs,
C.H. (1989) Improvement of Aerosol Distribution in Whole-Body Inhalation
Exposure Chambers. Inhal. Toxicol. 1: 153-166.
(8) Cheng,Y.S.; Moss, O.R. (1989) Inhalation Exposure Systems. In:
McClellan, R.O.; Henderson, R.F. ed. Concepts in Inhalation Toxicology.
New York, NY: Hemisphere Publishing Corp., 19-62.
(9) Cheng, Y.S.; Yeh, H.C.; Mauderly, J.L.; Mokler, B.V. (1984)
Characterization of Diesel Exhaust in a Chronic Inhalation Study. Am.
Ind. Hyg. Assoc. J. 45: 547-555.
(10) Gillum, D.R. (1982) Industrial Pressure Measurement. Research
Triangle Park, NC: Instrument Society of America.
(11) Hinners, R.G.; Burkart, J.K.; Malanchuk, M. (1979) Animal
Exposure Facility for Diesel Exhaust Studies.
(12) Kittelson, D.B.; Dolan, D.F. (1979) Diesel exhaust aerosols. In
Willeke, K. ed. Generation of Aerosols and Facilities for Exposure
Experiments. Ann Arbor, MI: Ann Arbor Science Publishers Inc., 337-360.
(13) Mokler, B.V.; Archibeque, F.A.; Beethe, R.L.; Kelly, C.P.J.;
Lopez, J.A.; Mauderly, J.L.; Stafford, D.L. (1984) Diesel Exhaust
Exposure System for Animal Studies. Fundamental and Applied Toxicology
4: 270-277.
(14) Moore, W.; et al. (1978) Preliminary finding on the Deposition
and Retention of Automotive Diesel Particulate in Rat Lungs. Proc. of
Annual Meeting of the Air Pollution Control Assn, 3, paper 78-33.7.
(15) Raabe, O.G., Bennick, J.E., Light, M.E., Hobbs, C.H., Thomas,
R.L., Tillery, M.I. (1973) An Improved Apparatus for Acute Inhalation
Exposure of Rodents to Radioactive Aerosols. Toxicol & Applied
Pharmaco.; 1973; 26: 264-273.
(16) Rao, G.N. (1986) Significance of Environmental Factors on the
Test System. In: Hoover, B.K.; Baldwin, J.K.; Uelner, A.F.; Whitmire,
C.E.; Davies, C.L.; Bristol, D.W. ed. Managing conduct and data quality
of toxicology studies. Raleigh, NC: Princeton Scientific Publishing Co.,
Inc.: 173-185.
(17) Spitzer, D.W. (1984) Industrial Flow Measurement. Research
Triangle Park, NC: Instrument Society of America.
(18) 40 CFR part 798, Health effects testing guidelines.
(19) 29 CFR part 1910, Occupational safety and health standards for
general industry.
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(20) Federal Register, 42 FR 26748, May 25, 1977.
[59 FR 33093, June 27, 1994, as amended at 61 FR 58746, Nov. 18, 1996;
61 FR 36512, July 11, 1996]